Arid
DOI10.1016/j.atmosres.2009.07.005
Chemical and strontium isotope characterization of rainwater at an urban site in Loess Plateau, Northwest China
Xu, Zhifang1; Li, Yushan2,3; Tang, Yang2,4; Han, Guilin4
通讯作者Xu, Zhifang
来源期刊ATMOSPHERIC RESEARCH
ISSN0169-8095
EISSN1873-2895
出版年2009
卷号94期号:3页码:481-490
英文摘要

Major ion concentrations and strontium isotopic ratios (Sr-87/Sr-86) were measured in rainwater samples collected at the urban site of Lanzhou, a city located on the Loess Plateau in the and and semiarid areas of northwest China. The rainwater samples possessed alkaline pH, at a reference level of 5.6, with a range of 6.82 to 8.28 and a volume-weighted mean (VWM) pH value of 7.70. The alkaline character of rainwater in Lanzhou is due to the result of neutralization caused by the alkaline soil dusts which contain large amount of CaCO3. It was observed that Ca2+ was the most abundant cation with a VWM value of 886 mu eq l(-1) (115-2184 mu eq l(-1)), accounting for 87.8% of the total cations. Without considering HCO3-, SO42- and NO3- were dominant among the anions, accounting for 64.2% and 23.0%, respectively, of the total measured anions. Using Na as an indicator of marine origin and Al for terrestrial inputs, the proportions of sea salt and non-sea-salt elements were estimated from elemental ratios. The precipitation in this region has typical continental characteristics. The Sr concentrations varied from 0.004 to 0.885 mu mol l(-1), and strontium isotopic ratios (Sr-87/Sr-86) lay in the range of 0.71025-0.71302, with an average of 0.71143. The Sr-87/Sr-86 ratios of Lanzhou rainwater are higher than that of seawater, which reflects contributions from the radiogenic Sr sources of the aerosols. The most suitable candidate for the source would be the soil dust originating from local and distant loess and desert areas. The Sr-87/Sr-86 ratios were used to characterize different sources of base cations in rainwater, suggesting that the samples could be interpreted in terms of combinations of at least three components: soil dust derived from the Loess Plateau and desert areas in northwest China (with Sr-87/Sr-86 similar to 0.7130), seawater (with (87)5r/Sr-86 similar to 0.70917), and anthropogenic inputs (With Sr-87/Sr-86 similar to 0.7103). The high Sr-87/Sr-86 ratio and Ca and Sr content in the rainwater from Lanzhou can be attributed to the dissolution of calcium carbonate in soil dust. (C) 2009 Elsevier B.V. All rights reserved.


英文关键词Major ions Strontium isotope Alkaline rain Lanzhou Loess Plateau
类型Article
语种英语
国家Peoples R China
收录类别SCI-E
WOS记录号WOS:000271336300011
WOS关键词MASSIF-CENTRAL FRANCE ; PRECIPITATION CHEMISTRY ; ACID-RAIN ; IONIC COMPOSITION ; HYDROGEOCHEMICAL IMPLICATIONS ; SEMIARID REGION ; TIBETAN PLATEAU ; WET DEPOSITION ; NORTHERN CHINA ; ATLANTIC OCEAN
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
来源机构中国科学院地质与地球物理研究所
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/159901
作者单位1.Chinese Acad Sci, Key Lab Engn Geomech, Inst Geol & Geophys, Beijing 100029, Peoples R China;
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China;
3.Chinese Acad Sci, Ecoenvironm Sci Res Ctr, Beijing 100085, Peoples R China;
4.Chinese Acad Sci, State Key Lab Environm Geochem, Inst Geochem, Guiyang 550002, Guizhou, Peoples R China
推荐引用方式
GB/T 7714
Xu, Zhifang,Li, Yushan,Tang, Yang,et al. Chemical and strontium isotope characterization of rainwater at an urban site in Loess Plateau, Northwest China[J]. 中国科学院地质与地球物理研究所,2009,94(3):481-490.
APA Xu, Zhifang,Li, Yushan,Tang, Yang,&Han, Guilin.(2009).Chemical and strontium isotope characterization of rainwater at an urban site in Loess Plateau, Northwest China.ATMOSPHERIC RESEARCH,94(3),481-490.
MLA Xu, Zhifang,et al."Chemical and strontium isotope characterization of rainwater at an urban site in Loess Plateau, Northwest China".ATMOSPHERIC RESEARCH 94.3(2009):481-490.
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