Arid
DOI10.1016/j.scitotenv.2008.03.041
Increases in ambient PCDD/F and PCB concentrations in Northern Taiwan during an Asian dust storm episode
Chi, Kai Hsien1; Hsu, Shih Chieh1; Wang, Sheng Hsiang2; Chang, Moo Been3
通讯作者Chi, Kai Hsien
来源期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
出版年2008
卷号401期号:1-3页码:100-108
英文摘要

In spring 2006, an Asian dust storm (ADS) that originated in the deserts of Mongolia and China eventually reached populated areas of East Asia, including Taiwan. The concentrations of total suspended particles (TSP), vapor/solid-phase dioxin-like compounds and metal content in atmospheric aerosols were monitored at two sampling sites in northern Taiwan during the ADS episode: one along the northern coast (Site A), and the other in Taipei city (Site B). The ADS swept across northern Taiwan from 13 March to 19 March, 2006. Data indicate that the atmospheric dibenzo-p-dioxin and dibenzofuran (PCDD/F, 32.2 to S2.5 fg-I-TEQ/m(3)) and polychlorinated biphenyl (PCB, 2.23 to 4.49 fg-TEQ(WHO)/m(3)) concentrations measured at the two sampling sites prior to the ADS episode were considerably lower than those measured in other Asian countries. However, measurements made at both sites on 13 and 18 March 2006 indicate that the atmospheric PCDD/F and PCB concentrations increased 2.5 and 3.2 times at Site A, and 2.1 and 1.9 times at Site B, respectively, during the ADS episode. The concentrations of aluminum (Al), potassium (K) and Titanium (Ti) in atmospheric aerosols were also found to increase about 2 to 5 times during this period. As no specific dioxin emission sources exist within nearly 20 km of Site A, the increase in PCDD/F and PCB concentrations observed there is likely to be related to the ADS from mainland China. Additionally, the amount of PCDD/Fs bound to suspended particles increased from 257-259 to 339-512 pg-I-TEQ/g-TSP during the ADS episode. The distribution of OCDD congener observed in Taipei city increased dramatically during the ADS episode, however, the distribution of PCB congener did not vary significantly. (c) 2008 Elsevier B.V. All rights reserved.


英文关键词dioxin sand storm aerosol ambient air long range transport
类型Article
语种英语
国家Japan ; Taiwan
收录类别SCI-E
WOS记录号WOS:000257690100011
WOS关键词INCINERATOR FLUE-GAS ; DIBENZO-P-DIOXINS ; OPTICAL-PROPERTIES ; CONGENER PATTERNS ; HONG-KONG ; AIR ; AEROSOLS ; KOREA ; ATMOSPHERE ; DEPOSITION
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/159148
作者单位1.Acad Sinica, Res Ctr Environm Changes, Tokyo 115, Japan;
2.Natl Cent Univ, Dept Atmospher Sci, Chungli 320, Taiwan;
3.Natl Cent Univ, Grad Inst Environm Engn, Chungli 320, Taiwan
推荐引用方式
GB/T 7714
Chi, Kai Hsien,Hsu, Shih Chieh,Wang, Sheng Hsiang,et al. Increases in ambient PCDD/F and PCB concentrations in Northern Taiwan during an Asian dust storm episode[J],2008,401(1-3):100-108.
APA Chi, Kai Hsien,Hsu, Shih Chieh,Wang, Sheng Hsiang,&Chang, Moo Been.(2008).Increases in ambient PCDD/F and PCB concentrations in Northern Taiwan during an Asian dust storm episode.SCIENCE OF THE TOTAL ENVIRONMENT,401(1-3),100-108.
MLA Chi, Kai Hsien,et al."Increases in ambient PCDD/F and PCB concentrations in Northern Taiwan during an Asian dust storm episode".SCIENCE OF THE TOTAL ENVIRONMENT 401.1-3(2008):100-108.
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