Arid
DOI10.5194/acp-8-3623-2008
The role of iron and black carbon in aerosol light absorption
Derimian, Y.1,4; Karnieli, A.1; Kaufman, Y. J.2; Andreae, M. O.3; Andreae, T. W.3; Dubovik, O.4; Maenhaut, W.5; Koren, I.6
通讯作者Derimian, Y.
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2008
卷号8期号:13页码:3623-3637
英文摘要

Iron is a major component of atmospheric aerosols, influencing the light absorption ability of mineral dust, and an important micronutrient that affects oceanic biogeochemistry. The regional distribution of the iron concentration in dust is important for climate studies however, this is difficult to obtain since it requires in-situ aerosol sampling or simulation of complex natural processes. Simultaneous studies of aerosol chemical composition and radiometric measurements of aerosol optical properties, which were performed in the Negev desert of Israel continuously for about eight years, suggest a potential for deriving a relationship between chemical composition and light absorption properties, in particular the spectral single-scattering albedo.


The two main data sets of the present study were obtained by a sun/sky radiometer and a stacked filter unit sampler that collects particles in coarse and fine size fractions. Analysis of chemical and optical data showed the presence of mixed dust and pollution aerosol in the study area, although their sources appear to be different. Spectral SSA showed an evident response to increased concentrations of iron, black carbon equivalent matter, and their mixing state. A relationship that relates the spectral SSA, the percentage of iron in total particulate mass., and the pollution components was derived. Results calculated, using this relationship, were compared with measurements from dust episodes in several locations around the globe. The comparison showed reasonable agreement between the calculated and the observed iron concentrations, and supported the validity of the suggested approach for the estimation of iron concentrations in mineral dust.


类型Article
语种英语
国家Israel ; USA ; Germany ; France ; Belgium
收录类别SCI-E
WOS记录号WOS:000257516800015
WOS关键词SUMMER AIRBORNE MEASUREMENTS ; SKY RADIANCE MEASUREMENTS ; EQUATORIAL PACIFIC-OCEAN ; OPTICAL-PROPERTIES ; SOUTHERN-OCEAN ; PHYTOPLANKTON BLOOM ; DUST AEROSOLS ; DESERT DUST ; AEGEAN SEA ; ACE-ASIA
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源机构Ben-Gurion University of the Negev
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/156546
作者单位1.Ben Gurion Univ Negev, Jacob Blaustein Inst Desert Res, IL-84105 Beer Sheva, Israel;
2.NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA;
3.Max Planck Inst Chem, D-55128 Mainz, Germany;
4.Univ Lille 1, CNRS, Opt Atmospher Lab, F-59655 Villeneuve Dascq, France;
5.Univ Ghent, Inst Nucl Sci, Dept Analyt Chem, B-9000 Ghent, Belgium;
6.Weizmann Inst Sci, Dept Environm Sci, IL-76100 Rehovot, Israel
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GB/T 7714
Derimian, Y.,Karnieli, A.,Kaufman, Y. J.,et al. The role of iron and black carbon in aerosol light absorption[J]. Ben-Gurion University of the Negev,2008,8(13):3623-3637.
APA Derimian, Y..,Karnieli, A..,Kaufman, Y. J..,Andreae, M. O..,Andreae, T. W..,...&Koren, I..(2008).The role of iron and black carbon in aerosol light absorption.ATMOSPHERIC CHEMISTRY AND PHYSICS,8(13),3623-3637.
MLA Derimian, Y.,et al."The role of iron and black carbon in aerosol light absorption".ATMOSPHERIC CHEMISTRY AND PHYSICS 8.13(2008):3623-3637.
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