Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.1021/es0505651 |
Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope | |
Ericksen, JA; Gustin, MS; Lindberg, SE; Olund, SD; Krabbenhoft, DP | |
通讯作者 | Gustin, MS |
来源期刊 | ENVIRONMENTAL SCIENCE & TECHNOLOGY
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ISSN | 0013-936X |
EISSN | 1520-5851 |
出版年 | 2005 |
卷号 | 39期号:20页码:8001-8007 |
英文摘要 | A solution containing Hg-198 in the form of HgCl2 was added to a 4 m(2) area of desert soils in Nevada, and soil Hg fluxes were measured using three dynamic flux chambers. There was an immediate release of Hg-198 after it was applied, and then emissions decreased exponentially. Within the first 6 h after the isotope was added to the soil, similar to 12 ng m(-2) of Hg-198 was emitted to the atmosphere, followed by a relatively steady flux of the isotope at 0.2 +/- 0.2 ng m(-2) h(-1) for the remainder of the experiment (62 days). Over this time, similar to 200 ng m(-2) or 2% of the Hg-198 isotope was emitted from the soil, and we estimate that similar to 6% of the isotope would be re-emitted in a year’s time. During the experiment, dry deposition of elemental Hg from the atmosphere was measured with an average deposition rate of 0.2 +/- 0.1 ng m(-2) h(-1). Emission of ambient Hg from the soil was observed after soil wetting with the isotope solution and after a storm event. However,the added moisture from the storm event did not affect 198Hg flux. Results suggest that in this desert environment, where there is limited precipitation, Hg deposited by wet processes is not readily re-emitted and that dry deposition of elemental Hg may be an important process. |
类型 | Article |
语种 | 英语 |
国家 | USA |
收录类别 | SCI-E |
WOS记录号 | WOS:000232758400038 |
WOS关键词 | ATMOSPHERIC MERCURY ; GAS-CHROMATOGRAPHY ; GASEOUS MERCURY ; EMISSIONS ; METHYLATION ; MOBILITY ; BEHAVIOR ; NEVADA |
WOS类目 | Engineering, Environmental ; Environmental Sciences |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
来源机构 | United States Geological Survey |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/148943 |
作者单位 | (1)Univ Nevada, Reno, NV 89557 USA;(2)US Geol Survey, Middleton, WI 53562 USA;(3)Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA |
推荐引用方式 GB/T 7714 | Ericksen, JA,Gustin, MS,Lindberg, SE,et al. Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope[J]. United States Geological Survey,2005,39(20):8001-8007. |
APA | Ericksen, JA,Gustin, MS,Lindberg, SE,Olund, SD,&Krabbenhoft, DP.(2005).Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope.ENVIRONMENTAL SCIENCE & TECHNOLOGY,39(20),8001-8007. |
MLA | Ericksen, JA,et al."Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope".ENVIRONMENTAL SCIENCE & TECHNOLOGY 39.20(2005):8001-8007. |
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