Arid
DOI10.1021/es0505651
Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope
Ericksen, JA; Gustin, MS; Lindberg, SE; Olund, SD; Krabbenhoft, DP
通讯作者Gustin, MS
来源期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN0013-936X
EISSN1520-5851
出版年2005
卷号39期号:20页码:8001-8007
英文摘要

A solution containing Hg-198 in the form of HgCl2 was added to a 4 m(2) area of desert soils in Nevada, and soil Hg fluxes were measured using three dynamic flux chambers. There was an immediate release of Hg-198 after it was applied, and then emissions decreased exponentially. Within the first 6 h after the isotope was added to the soil, similar to 12 ng m(-2) of Hg-198 was emitted to the atmosphere, followed by a relatively steady flux of the isotope at 0.2 +/- 0.2 ng m(-2) h(-1) for the remainder of the experiment (62 days). Over this time, similar to 200 ng m(-2) or 2% of the Hg-198 isotope was emitted from the soil, and we estimate that similar to 6% of the isotope would be re-emitted in a year’s time. During the experiment, dry deposition of elemental Hg from the atmosphere was measured with an average deposition rate of 0.2 +/- 0.1 ng m(-2) h(-1). Emission of ambient Hg from the soil was observed after soil wetting with the isotope solution and after a storm event. However,the added moisture from the storm event did not affect 198Hg flux. Results suggest that in this desert environment, where there is limited precipitation, Hg deposited by wet processes is not readily re-emitted and that dry deposition of elemental Hg may be an important process.


类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:000232758400038
WOS关键词ATMOSPHERIC MERCURY ; GAS-CHROMATOGRAPHY ; GASEOUS MERCURY ; EMISSIONS ; METHYLATION ; MOBILITY ; BEHAVIOR ; NEVADA
WOS类目Engineering, Environmental ; Environmental Sciences
WOS研究方向Engineering ; Environmental Sciences & Ecology
来源机构United States Geological Survey
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/148943
作者单位(1)Univ Nevada, Reno, NV 89557 USA;(2)US Geol Survey, Middleton, WI 53562 USA;(3)Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA
推荐引用方式
GB/T 7714
Ericksen, JA,Gustin, MS,Lindberg, SE,et al. Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope[J]. United States Geological Survey,2005,39(20):8001-8007.
APA Ericksen, JA,Gustin, MS,Lindberg, SE,Olund, SD,&Krabbenhoft, DP.(2005).Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope.ENVIRONMENTAL SCIENCE & TECHNOLOGY,39(20),8001-8007.
MLA Ericksen, JA,et al."Assessing the potential for re-emission of mercury deposited in precipitation from arid soils using a stable isotope".ENVIRONMENTAL SCIENCE & TECHNOLOGY 39.20(2005):8001-8007.
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