Arid
DOI10.1029/2003JD004239
Aerosol chemical, physical, and radiative characteristics near a desert source region of northwest China during ACE-Asia
Xu, J; Bergin, MH; Greenwald, R; Schauer, JJ; Shafer, MM; Jaffrezo, JL; Aymoz, G
通讯作者Xu, J
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2004
卷号109期号:D19
英文摘要

The Gobi desert in northwest China is an important source of mineral aerosols over both eastern Asia and the northern Pacific Ocean. In order to determine the chemical, physical, and radiative properties of aerosols originating from the Gobi desert source region, field measurements were performed in Yulin, China, in April 2001 as part of the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia) campaign. The means and standard deviations of the measured aerosol light absorption coefficient sigma(ap), scattering coefficient sigma(sp), and single-scattering albedo omega are 6 Mm(-1) (11 Mm(-1)), 158 Mm(-1) (193 Mm(-1)), and 0.95 (0.05), respectively. A clear diurnal pattern is observed in both sigma(ap) and sigma(sp), resulting from diurnal changes in the mixing height as well as from local combustion sources in the morning and dust sources in the afternoon. Two distinct populations of aerosol mass scattering efficiencies E-scat_2.5, one for aerosols dominated by desert dust (similar to1.0 m(2) g(-1)) and the other for aerosols composed primarily of local pollutants (similar to3.0 m(2) g(-1)), are observed. During the field study there were three significant dust events that occurred for, on average, several days at a time. The most significant dust storm resulted in a 24-hour-average PM2.5 concentration ( mass concentration of particles having aerodynamic diameters less than 2.5 mum) of 453 mug m(-3) and a peak sigma(sp) of 2510 Mm(-1) on 8 April. The mean PM2.5 mass concentration during the dust storm periods is approximately 169 mug m(-3), about 4 times greater than the mean value of 44 mug m(-3) observed during local pollution periods. When local pollution is the dominant source of fine particulate mass, organic matter ( OM) is the major chemical component, contributing 41% to the PM2.5 mass, followed by crustal material (29%), sulfate (17%), and elemental carbon (EC) (13%). During sand storm periods, similar to51% of PM2.5 mass is crustal material, followed by CO32- (11%) and OM (9.5%). The element enrichment factors indicate that coal combustion, biomass burning, and mobile source emissions are important local pollution sources. Overall, our results indicate that in addition to dust, local pollution also has a significant influence on aerosol properties in the region.


英文关键词aerosol dust ACE-Asia
类型Article
语种英语
国家USA ; France
收录类别SCI-E
WOS记录号WOS:000223336800005
WOS关键词LONG-RANGE TRANSPORT ; YANGTZE DELTA REGION ; MINERAL DUST ; OPTICAL-PROPERTIES ; ELEMENTAL CARBON ; NORTHERN FINLAND ; PACIFIC-OCEAN ; LOESS PLATEAU ; YELLOW SAND ; VARIABILITY
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
来源机构Desert Research Institute
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/147374
作者单位(1)Desert Res Inst, Div Atmospher Sci, Las Vegas, NV 89119 USA;(2)Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA;(3)Univ Wisconsin, Dept Civil & Environm Engn, Environm Chem & Technol Program, Madison, WI 53706 USA;(4)Ecole Natl Super Electrochim & Electrome Grenoble, Thermodynam & Physicochim Met Lab, CNRS, Lab Glaciol & Geophys Environm, F-38402 St Martin Dheres, France
推荐引用方式
GB/T 7714
Xu, J,Bergin, MH,Greenwald, R,et al. Aerosol chemical, physical, and radiative characteristics near a desert source region of northwest China during ACE-Asia[J]. Desert Research Institute,2004,109(D19).
APA Xu, J.,Bergin, MH.,Greenwald, R.,Schauer, JJ.,Shafer, MM.,...&Aymoz, G.(2004).Aerosol chemical, physical, and radiative characteristics near a desert source region of northwest China during ACE-Asia.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,109(D19).
MLA Xu, J,et al."Aerosol chemical, physical, and radiative characteristics near a desert source region of northwest China during ACE-Asia".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 109.D19(2004).
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