Arid
DOI10.5194/acp-4-1201-2004
Aerosol-ozone correlations during dust transport episodes
Bonasoni, P; Cristofanelli, P; Calzolari, F; Bonafe, U; Evangelisti, F; Stohl, A; Sajani, SZ; van Dingenen, R; Colombo, T; Balkanski, Y
通讯作者Bonasoni, P
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2004
卷号4页码:1201-1215
英文摘要

Its location in the Mediterranean region and its physical characteristics render Mt. Cimone (44degrees 11’ N, 10degrees 42’ E), the highest peak of the Italian northern Apennines (2165 m asl), particularly suitable to study the transport of air masses from the north African desert area to Europe. During these northward transports 12 dust events were registered in measurements of the aerosol concentration at the station during the period June - December 2000, allowing the study of the impact of mineral dust transports on free tropospheric ozone concentrations, which were also measured at Mt. Cimone. Three-dimensional backward trajectories were used to determine the air mass origin, while TOMS Aerosol Index data for the Mt. Cimone area were used to confirm the presence of absorbing aerosol over the measurement site.


A trajectory statistical analysis allowed identifying the main source areas of ozone and aerosols. The analysis of these back trajectories showed that central Europe and north and central Italy are the major pollution source areas for ozone and fine aerosol, whereas the north African desert regions were the most important source areas for coarse aerosol and low ozone concentrations. During dust events, the Mt. Cimone mean volume concentration for coarse particles was 6.18 mum(3)/cm(3) compared to 0.63 mum(3)/cm(3) in dust-free conditions, while the ozone concentrations were 4% to 21% lower than the monthly mean background values. Our observations show that surface ozone concentrations were lower than the background values in air masses coming from north Africa, and when these air masses were also rich in coarse particles, the lowest ozone values were registered. Moreover, preliminary results on the possible impact of the dust events on PM10 and ozone values measured in Italian urban and rural areas showed that during the greater number of the considered dust events, significant PM10 increases and ozone decreases have occurred in the Po valley.


类型Article
语种英语
国家Italy ; USA ; France
收录类别SCI-E
WOS记录号WOS:000223066300002
WOS关键词ULTRAVIOLET-RADIATION ; AIR-POLLUTANTS ; TRAJECTORY STATISTICS ; GLOBAL TROPOSPHERE ; TOMS OBSERVATIONS ; PHOTOLYSIS RATES ; FORECAST MODEL ; NORTH-ATLANTIC ; MINERAL DUST ; MT. CIMONE
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/146262
作者单位(1)CNR, Inst Atmospher Sci & Climate, I-40129 Bologna, Italy;(2)Univ Colorado, NOAA, Aeron Lab, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA;(3)Agenzia Reg Prevenz & Ambiente Emilia Romagna, Struttura Temat Epidemiol Ambientale, Modena, Italy;(4)Commiss European Communities, Joint Res Ctr, I-21020 Ispra, Italy;(5)Ufficio Gen Meteorol, Prat Mare, Rome, Italy;(6)Lab Sci Climat & Environm, Gif Sur Yvette, France
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GB/T 7714
Bonasoni, P,Cristofanelli, P,Calzolari, F,et al. Aerosol-ozone correlations during dust transport episodes[J],2004,4:1201-1215.
APA Bonasoni, P.,Cristofanelli, P.,Calzolari, F.,Bonafe, U.,Evangelisti, F.,...&Balkanski, Y.(2004).Aerosol-ozone correlations during dust transport episodes.ATMOSPHERIC CHEMISTRY AND PHYSICS,4,1201-1215.
MLA Bonasoni, P,et al."Aerosol-ozone correlations during dust transport episodes".ATMOSPHERIC CHEMISTRY AND PHYSICS 4(2004):1201-1215.
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