Arid
DOI10.1029/2002JD003290
Large-scale ozone and aerosol distributions, air mass characteristics, and ozone fluxes over the western Pacific Ocean in late winter/early spring
Browell, EV; Fenn, MA; Butler, CF; Grant, WB; Brackett, VG; Hair, JW; Avery, MA; Newell, RE; Hu, YL; Fuelberg, HE; Jacob, DJ; Anderson, BE; Atlas, EL; Blake, DR; Brune, WH; Dibb, JE; Fried, A; Heikes, BG; Sachse, GW; Sandholm, ST; Singh, HB; Talbot, RW; Vay, SA; Weber, RJ; Bartlett, KB
通讯作者Browell, EV
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2003
卷号108期号:D20
英文摘要

[1] Large-scale measurements of ozone (O-3) and aerosol distributions were made from the NASA DC-8 aircraft during the Transport and Chemical Evolution over the Pacific (TRACE-P) field experiment conducted in February-April 2001. Remote measurements were made with an airborne lidar to provide O-3 and multiple-wavelength aerosol backscatter profiles from near the surface to above the tropopause along the flight track. In situ measurements of O-3, aerosols, and a wide range of trace gases were made onboard the DC-8. Five-day backward trajectories were used in conjunction with the O-3 and aerosol distributions on each flight to indicate the possible origin of observed air masses, such as from biomass burning regions, continental pollution, desert regions, and oceanic regions. Average latitudinal O-3 and aerosol scattering ratio distributions were derived from all flights west of 150degreesE, and these distributions showed the average latitude and altitude dependence of different dynamical and chemical processes in determining the atmospheric composition over the western Pacific. TRACE-P (TP) showed an increase in the average latitudinal distributions of both O-3 and aerosols compared to PEM-West B (PWB), which was conducted in February-March 1994. O-3, aerosol, and potential vorticity levels were used to identify nine air mass types and quantify their frequency of occurrence as a function of altitude. This paper discusses the characteristics of the different air mass types encountered during TP and compares them to PWB. These results confirmed that most of the O-3 increase in TP was due to photochemistry. The average latitudinal eastward O-3 flux in the western Pacific during TP was found to peak near 32degreesN with a total average O-3 flux between 14 and 46degreesN of 5.2 Tg/day. The eastward total CO flux was calculated to be 2.2 Tg-C/day with -6% estimated from Asia. The Asian flux of CO2 and CH4 was estimated at 4.9 and 0.06 Tg-C/day.


英文关键词ozone aerosols fluxes air mass characteristics western Pacific TRACE-P
类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:000185361800002
WOS关键词LONG-RANGE TRANSPORT ; EXPLORATORY MISSION-WEST ; EAST-ASIA ; NORTH-AMERICA ; PEM-WEST ; CHEMICAL CHARACTERISTICS ; CONTINENTAL OUTFLOW ; TROPOSPHERIC OZONE ; DIAL MEASUREMENTS ; CARBON-MONOXIDE
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/145193
作者单位(1)NASA, Langley Res Ctr, Hampton, VA 23681 USA;(2)Sci Applicat Int Corp, Hampton, VA USA;(3)MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA USA;(4)Florida State Univ, Dept Meteorol, Tallahassee, FL 32306 USA;(5)Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA;(6)Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA;(7)Univ Calif Irvine, Dept Chem, Irvine, CA 92717 USA;(8)Penn State Univ, Dept Meteorol, University Pk, PA 16802 USA;(9)Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA;(10)Univ Rhode Isl, Grad Sch Oceanog, Narragansett, RI 02882 USA;(11)Georgia Inst Technol, Dept Earth & Atmospher Sci, Atlanta, GA 30332 USA;(12)NASA, Ames Res Ctr, Moffett Field, CA 94035 USA
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Browell, EV,Fenn, MA,Butler, CF,et al. Large-scale ozone and aerosol distributions, air mass characteristics, and ozone fluxes over the western Pacific Ocean in late winter/early spring[J],2003,108(D20).
APA Browell, EV.,Fenn, MA.,Butler, CF.,Grant, WB.,Brackett, VG.,...&Bartlett, KB.(2003).Large-scale ozone and aerosol distributions, air mass characteristics, and ozone fluxes over the western Pacific Ocean in late winter/early spring.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,108(D20).
MLA Browell, EV,et al."Large-scale ozone and aerosol distributions, air mass characteristics, and ozone fluxes over the western Pacific Ocean in late winter/early spring".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 108.D20(2003).
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