Arid
DOI10.1029/2002JD002807
Tropospheric aerosols in the Mediterranean: 2. Radiative effects through model simulations and measurements
Meloni, D; di Sarra, A; DeLuisi, J; Di Iorio, T; Fiocco, G; Junkermann, W; Pace, G
通讯作者Meloni, D
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
出版年2003
卷号108期号:D10
英文摘要

[1] The radiative effects of tropospheric aerosols at the island of Lampedusa, in the Mediterranean, have been investigated by comparing measurements and results from a radiative transfer model. The model was used to reproduce the measured ultraviolet irradiance spectra (286.5 - 363 nm) in three cases of cloud-free conditions in May 1999, allowing the estimation of the aerosol properties and of the direct radiative forcing. Observations show very different aerosol loading and distribution, connected to the different origins of the air masses: low aerosol optical depths are associated with air masses from North Atlantic/Europe ( 25 and 27 May), and larger particles up to 7 km altitude and larger optical depths are observed for mineral dust coming from the Saharan region ( 18 May). The detailed description of the atmospheric structure and composition was used to initialize the radiative transfer model. The estimated single-scattering albedo and asymmetry parameter at 500 nm for the desert dust are in the range 0.73 - 0.84 and in the range 0.75 - 0.79, respectively. Radiative transfer calculations show that differences of the surface ultraviolet irradiance larger than 10% may arise from the lack of a detailed knowledge of the aerosol size distribution. Aerosol may also increase or reduce the absorption effectiveness of tropospheric ozone, depending on the characteristics of the particles. Estimates of the direct aerosol radiative forcing in the spectral range 300 - 800 nm at the surface and at the top of the atmosphere (TOA) were also derived. At the surface, aerosols produce a decrease of the instantaneous downward irradiance with respect to an aerosol-free atmosphere by 70.8, 37.2, and 39.1 W m(-2), for 18 May ( the aerosol optical depth is 0.511 at 415 nm), 25 (0.165) and 27 (0.224), respectively. The radiative forcing per unit optical depth at the surface is largest for aerosol of continental/ marine origin, transported from North. The forcing at the TOA is negative, thus producing a cooling, in the desert dust case, and close to zero or positive for aerosol originating from North.


英文关键词aerosol radiative forcing atmospheric ozone dust atmospheric transmission
类型Article
语种英语
国家Italy ; USA ; Germany
收录类别SCI-E
WOS记录号WOS:000183303100004
WOS关键词SOLAR ULTRAVIOLET-RADIATION ; TROPICAL INDIAN-OCEAN ; UV-B RADIATION ; OPTICAL-DEPTH ; PHOTOCHEMICAL ACTIVITY ; EARTHS SURFACE ; MINERAL DUST ; OZONE ; UNCERTAINTIES ; IRRADIANCES
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/145166
作者单位(1)Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy;(2)Ente Nuove Tecnol Energia Ambiente ENEA, Climate Lab, CLIM OSS, I-00060 Santa Maria Di Galeria, Italy;(3)NOAA, Surface Radiat Res Branch, Boulder, CO 80303 USA;(4)Forschungszentrum Karlsruhe, Inst Meteorol & Climate Res, IMK, IFU, D-8100 Garmisch Partenkirchen, Germany
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GB/T 7714
Meloni, D,di Sarra, A,DeLuisi, J,et al. Tropospheric aerosols in the Mediterranean: 2. Radiative effects through model simulations and measurements[J],2003,108(D10).
APA Meloni, D.,di Sarra, A.,DeLuisi, J.,Di Iorio, T.,Fiocco, G.,...&Pace, G.(2003).Tropospheric aerosols in the Mediterranean: 2. Radiative effects through model simulations and measurements.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,108(D10).
MLA Meloni, D,et al."Tropospheric aerosols in the Mediterranean: 2. Radiative effects through model simulations and measurements".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 108.D10(2003).
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