Arid
DOI10.1029/96GL00778
Aerosol dynamics in the equatorial Pacific Marine boundary layer: Microphysics, diurnal cycles and entrainment
Clarke, AD; Li, Z; Litchy, M
通讯作者Clarke, AD
来源期刊GEOPHYSICAL RESEARCH LETTERS
ISSN0094-8276
出版年1996
卷号23期号:7页码:733-736
英文摘要

During July-August of 1994 we measured the size-resolved physicochemical properties of aerosol particles at Christmas Island in the equatorial Pacific. In spite of rapid diurnal conversion of dimethylsulfide (DMS) to sulfur dioxide (SO2) we found no evidence for new particle production in the marine boundary layer (MBL) and more than 95% of all particles were consistently larger than 0.02 mu m diameter, indicating an aged aerosol. The submicrometer aerosol number (size-distribution) was bimodal with peaks near 0.05 mu m and 0.2 mu m particle diameter (D-p) and had a cloud-processed intermode minimum at about 0.09 mu m that varied in phase with diurnal changes in ozone concentration This suggests that the number distribution for condensation nuclei (CN) arid cloud condensation nuclei (CCN) was maintained by a quasi-equilibrium between entrainment (estimated to be 0.6 +/- 0.2 cm s(-1)) from sources aloft and processes in the MBL. This implies a replenishment timescale for nuclei of about 2 and 4 days for this region. The stability of the distribution and the 0.09 mu m cloud processed minima suggests trade wind cumulus supersaturations near 0.35% and updrafts near 1 m s(-1).


类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:A1996UD38000010
WOS关键词CONDENSATION NUCLEI ; NUCLEATION
WOS类目Geosciences, Multidisciplinary
WOS研究方向Geology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/132775
作者单位(1)UNIV HAWAII,DEPT METEOROL,HONOLULU,HI 96822
推荐引用方式
GB/T 7714
Clarke, AD,Li, Z,Litchy, M. Aerosol dynamics in the equatorial Pacific Marine boundary layer: Microphysics, diurnal cycles and entrainment[J],1996,23(7):733-736.
APA Clarke, AD,Li, Z,&Litchy, M.(1996).Aerosol dynamics in the equatorial Pacific Marine boundary layer: Microphysics, diurnal cycles and entrainment.GEOPHYSICAL RESEARCH LETTERS,23(7),733-736.
MLA Clarke, AD,et al."Aerosol dynamics in the equatorial Pacific Marine boundary layer: Microphysics, diurnal cycles and entrainment".GEOPHYSICAL RESEARCH LETTERS 23.7(1996):733-736.
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