Arid
DOI10.2134/jeq1995.00472425002400060004x
CONTAMINANT RELEASE FROM SOLIDIFIED RADIOACTIVE-WASTES BURIED IN UNSATURATED SEDIMENTS - LYSIMETER STUDY
JONES, TL; SERNE, RJ
通讯作者JONES, TL
来源期刊JOURNAL OF ENVIRONMENTAL QUALITY
ISSN0047-2425
出版年1995
卷号24期号:6页码:1063-1073
英文摘要

A lysimeter facility has been used since 1984 to monitor the leaching of buried waste forms under natural, arid conditions. The facility includes 10 bare-soil lysimeters (183 cm diam, by 305 cm deep) containing buried waste forms solidified with Portland III cement, masonry cement, bitumen, and vinyl-ester styrene. From 1984 through 1992, an average of 45 cm of water (27% of area precipitation) have leached through the lysimeters. To date, tritium, Co-60, and Cs-137 have been identified in the lysimeter leachate samples. From 1984 through 1992, >4000 mu Ci of tritium, representing 76 and 71% of inventory (not decay corrected), have been leached from the two waste forms containing tritium. Cobalt-60 (0.1% of original Co inventories) has been found in the leachate from each of all six of the waste forms that originally contained >1 mCi of inventory, Mobile Co is believed to be chelated with organic compounds, such as EDTA, present in the waste. Trace amounts of Cs-137 have occasionally been identified in leachate from two waste forms since 1991. Qualitatively, the held leaching results confirm laboratory studies, suggesting that tritium is readily leached from cement, and that Co-60 is generally leached more from cement than from vinyl-ester styrene. These data suggest that empirical source-term models should predict leaching based on the amount of water flowing past the waste form, not based on time.


类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:A1995TF75800003
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
来源机构New Mexico State University
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/131607
作者单位(1)PACIFIC NW LAB, DEPT GEOSCI, RICHLAND, WA 99352 USA
推荐引用方式
GB/T 7714
JONES, TL,SERNE, RJ. CONTAMINANT RELEASE FROM SOLIDIFIED RADIOACTIVE-WASTES BURIED IN UNSATURATED SEDIMENTS - LYSIMETER STUDY[J]. New Mexico State University,1995,24(6):1063-1073.
APA JONES, TL,&SERNE, RJ.(1995).CONTAMINANT RELEASE FROM SOLIDIFIED RADIOACTIVE-WASTES BURIED IN UNSATURATED SEDIMENTS - LYSIMETER STUDY.JOURNAL OF ENVIRONMENTAL QUALITY,24(6),1063-1073.
MLA JONES, TL,et al."CONTAMINANT RELEASE FROM SOLIDIFIED RADIOACTIVE-WASTES BURIED IN UNSATURATED SEDIMENTS - LYSIMETER STUDY".JOURNAL OF ENVIRONMENTAL QUALITY 24.6(1995):1063-1073.
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