Arid
DOI10.1016/0883-2927(93)90075-R
RADIONUCLIDES IN-GROUND WATER OF THE CARSON RIVER BASIN, WESTERN NEVADA AND EASTERN CALIFORNIA, USA
THOMAS, JM; WELCH, AH; LICO, MS; HUGHES, JL; WHITNEY, R
通讯作者THOMAS, JM
来源期刊APPLIED GEOCHEMISTRY
ISSN0883-2927
出版年1993
卷号8期号:5页码:447-471
英文摘要

Ground water is the main source of domestic and public supply in the Carson River Basin. Ground water originates as precipitation primarily in the Sierra Nevada in the western part of Carson and Eagle Valleys, and flows down gradient in the direction of the Carson River through Dayton and Churchill Valleys to a terminal sink in the Carson Desert. Because radionuclides dissolved in ground water can pose a threat to human health, the distribution and sources of several naturally occurring radionuclides that contribute to gross-alpha and gross-beta activities in the study area were investigated. Generally, alpha and beta activities and U concentration increase from the up-gradient to down-gradient hydrographic areas of the Carson River Basin, whereas Rn-222 concentration decreases. Both Ra-226 and Ra-228 concentrations are similar throughout the study area. Alpha and beta activities and U concentration commonly exceed 100 pCi/l in the Carson Desert at the distal end of the flow system. Radon-222 commonly exceeds 2,000 pCi/l in the western part of Carson and Eagle Valleys adjacent to the Sierra Nevada. Radium-226 and Ra-228 concentrations are <5 pCi/l. Four ground water samples were analyzed for Po-210 and one sample contained a high concentration of 21 pCi/l. Seven samples were analyzed for Pb-210; six contained <3 pCiA and one contained 12 pCi/l. Thorium-230 was detected at concentrations of 0.15 and 0.20 pCi/l in two of four samples.


Alpha-emitting radionuclides in the ground water originated from the dissolution of U-rich granitic rocks in the Sierra Nevada by CO2, oxygenated water. Dissolution of primary minerals, mainly titanite (sphene) in the granitic rocks, releases U to the water. Dissolved U is probably removed from the water by adsorption on Fe- and Mn-oxide coatings on fracture surfaces and fine-grained sediment, by adsorption on organic matter, and by coprecipitation with Fe and Mn oxides. These coated sediments are transported throughout the basin by fluvial processes. Thus, U is transported as dissolved and adsorbed species. A rise in the water table in the Carson Desert because of irrigation has resulted in the oxidation of U-rich organic matter and dissolution of U-bearing coatings on sediments, producing unusually high U concentration in the ground water.


Alpha activity in the ground water is almost entirely from the decay of U dissolved in the water. Beta activity in ground water samples is primarily from the decay of K-40 dissolved in the water and ingrowth of U-238 progeny in the sample before analysis. Approximately one-half of the measured beta activity may not be present in ground water in the aquifer, but instead is produced in the sample after collection and before analysis. Potassium-40 is primarily from the dissolution of K-containing minerals, probably K-feldspar and biotite. Radon-222 is primarily from the decay of Ra-226 in the aquifer materials. Radium in the ground water is thought to be mainly from alpha recoil associated with the decay of Th in the aquifer material. Some Ra may be from dissolution (or desorption) of Ra-rich coatings on sediments.


类型Article
语种英语
收录类别SCI-E
WOS记录号WOS:A1993LV29800003
WOS类目Geochemistry & Geophysics
WOS研究方向Geochemistry & Geophysics
来源机构United States Geological Survey
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/128496
推荐引用方式
GB/T 7714
THOMAS, JM,WELCH, AH,LICO, MS,et al. RADIONUCLIDES IN-GROUND WATER OF THE CARSON RIVER BASIN, WESTERN NEVADA AND EASTERN CALIFORNIA, USA[J]. United States Geological Survey,1993,8(5):447-471.
APA THOMAS, JM,WELCH, AH,LICO, MS,HUGHES, JL,&WHITNEY, R.(1993).RADIONUCLIDES IN-GROUND WATER OF THE CARSON RIVER BASIN, WESTERN NEVADA AND EASTERN CALIFORNIA, USA.APPLIED GEOCHEMISTRY,8(5),447-471.
MLA THOMAS, JM,et al."RADIONUCLIDES IN-GROUND WATER OF THE CARSON RIVER BASIN, WESTERN NEVADA AND EASTERN CALIFORNIA, USA".APPLIED GEOCHEMISTRY 8.5(1993):447-471.
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