Arid
DOI10.1021/acs.iecr.5b04927
Photocatalytic Disinfection and Removal of Emerging Pollutants from Effluents of Biological Wastewater Treatments, Using a Newly Developed Large-Scale Solar Simulator
Philippe, Karine K.; Timmers, Ruud; van Grieken, Rafael; Marugan, Javier
通讯作者Marugan, Javier
来源期刊INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN0888-5885
出版年2016
卷号55期号:11页码:2952-2958
英文摘要

The reuse of sewage water treatment is becothing a priority, especially in arid regions, where water is scarce. However, there is increasing concern about the presence of emerging micropollutants refractory to the conventional treatments in wastewater treatment plants. Solar TiO2 heterogeneous photocatalysis provides a valuable alternative for the simultaneous oxidation of chemical and inactivation of microorganisms. However, the variability of solar irradiance hinders the study of the process under controlled ultraviolet (UV) irradiance. This work reports the development of an innovative solar simulator and its validation against the use of natural sunlight in photocatalytic disinfection applications with simultaneous removal of emerging contaminants. The significant impact of osmotic and mechanical stress on the viability of E. coli bacteria was confirmed. UV irradiance and total-to-illuminated volume ratio showed no impact on the dependence of the bacteria inactivation kinetics on the energy accumulated in the system, indicating that the possible existence of dark repair mechanisms can be neglected within the studied irradiance range (20-60 W m(-2).). Average results show that after an accumulated energy of 3 kJ L-1, 5 logarithmic units (5-logs) of E. coli bacteria are inactivated, whereas a removal efficiency of >80% is achieved for the micropollutants.


类型Article
语种英语
国家Spain
收录类别SCI-E
WOS记录号WOS:000372854600005
WOS关键词TIO2 PHOTOCATALYSIS ; ESCHERICHIA-COLI ; DRINKING-WATER ; E. COLI ; INACTIVATION ; OXIDATION ; UV ; INTENSITY ; PHARMACEUTICALS ; MICROORGANISMS
WOS类目Engineering, Chemical
WOS研究方向Engineering
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/193589
作者单位Univ Rey Juan Carlos, ESCET, Dept Chem & Environm Technol, C Tulipan S-N, Mostoles 28933, Spain
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GB/T 7714
Philippe, Karine K.,Timmers, Ruud,van Grieken, Rafael,et al. Photocatalytic Disinfection and Removal of Emerging Pollutants from Effluents of Biological Wastewater Treatments, Using a Newly Developed Large-Scale Solar Simulator[J],2016,55(11):2952-2958.
APA Philippe, Karine K.,Timmers, Ruud,van Grieken, Rafael,&Marugan, Javier.(2016).Photocatalytic Disinfection and Removal of Emerging Pollutants from Effluents of Biological Wastewater Treatments, Using a Newly Developed Large-Scale Solar Simulator.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,55(11),2952-2958.
MLA Philippe, Karine K.,et al."Photocatalytic Disinfection and Removal of Emerging Pollutants from Effluents of Biological Wastewater Treatments, Using a Newly Developed Large-Scale Solar Simulator".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 55.11(2016):2952-2958.
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